Enhanced infrared-to-visible upconversion imaging via metasurface–lanthanide nanoparticle hybrid screens
Abstract
Abstract Accessing the rich information carried by infrared light typically relies on bulky, complex optoelectronic systems. Lanthanide-based upconverting nanoparticles (UCNPs) offer a compelling alternative by converting infrared light into visible photons through nonlinear anti-Stokes processes. However, achieving strong upconversion under the low excitation intensities relevant to infrared vision remains challenging, motivating strategies to enhance light–matter interaction. Here, we demonstrate enhanced infrared-to-visible upconversion imaging enabled by integrating alloyed Yb/Er UCNPs with a resonant dielectric metasurface. The metasurface supports an optical resonance aligned with the UCNP excitation band, leading to over three orders of magnitude enhancement in upconversion emission. Crucially, flat-band angular dispersion of this resonance enables uniform enhancement across incident angles relevant to imaging, thereby preserving spatial frequency content and yielding sharp, high-contrast images. In light of ongoing advances in lanthanide-based materials, this metasurface–UCNP hybrid screen provides a promising platform for compact, detector-free, and scalable infrared imaging technologies based on optical upconversion.
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Authors: Nima Sefidmooye Azar, Matthew Parry, Xiao Qi, Changhwan Lee, Wendy S. L. Lee, Benjamin Russell, Wei Luo, Robert W. de Gille, Damian Nelson, Sivacarendran Balendhran, Jiajun Meng, Henry Tan, Gus O. Bonin, Duk‐Yong Choi, P. James Schuck, Emory M. Chan, Bruce E. Cohen, Dragomir N. Neshev, Kenneth B. Crozier
Institutions: Columbia University, The University of Melbourne, Korea Advanced Institute of Science and Technology, Australian National University, Lawrence Berkeley National Laboratory, ARC Centre of Excellence for Transformative Meta-Optical Systems