Suppression of spectral gap and flat bands on a cuprate superconductor side-surface
Abstract
Abstract Side surfaces of cuprate superconductors are expected to display a suppressed d -wave order parameter and zero-energy topological flat bands with a large density of states, making them susceptible to symmetry broken orders. Yet such surfaces have never been investigated with momentum-resolved, surface-sensitive probes, because high-temperature superconductors rarely cleave along them. Using focused-ion-beam milling to define a controlled breaking point, we expose pristine (110) side surfaces of overdoped La 2− x Sr x CuO 4 ( x = 0.22) suitable for angle-resolved photoemission. We do not resolve an opening or closing of a superconducting spectral gap within our energy resolution ( ~ 4 meV), in agreement with theoretical predictions. Surprisingly, the expected zero-energy flat band peak is also suppressed, despite the high topographic quality of the surface. Self-consistent Bogoliubov–de Gennes calculations show that the measured geometric roughness of the cleaved surface is too weak to eliminate these modes. The calculations further demonstrate that bulk inhomogeneities characteristic of high-temperature superconductors, modelled as moderate Anderson-type disorder, can broaden the flat-band states beyond detectability. Our results provide the first momentum-resolved view of the electronic structure on a cuprate side surface and identify disorder as a plausible mechanism obscuring the spectroscopic signatures of the predicted flat-band states.
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Authors: Gabriele Domaine, Mihir Date, S. K. Y. Dufresne, Natalie Lehmann, Daiyu Geng, T. Kurosawa, Amit Kumar, Jiaju Wang, Tianlun Yu, Chien-Ching Chang, Swosti P. Sarangi, Ding Pei, Yiran Liu, J. Küspert, Shigemi Terakawa, Markel Pardo Almanza, Jiabao Yang, I. Biało, M. D. Watson, Timur K. Kim, S. M. Hayden, Kritika Singh, Banabir Pal, M. Minola, J. F. Chang, N. Momono, Migaku Oda, S. Parkin, Andreas P. Schnyder, Niels B. M. Schröter
Institutions: University of Bristol, The University of Osaka, Hokkaido University, University of Zurich, Martin Luther University Halle-Wittenberg, Helmholtz-Zentrum Hereon, Synchrotron SOLEIL, Max Planck Institute of Microstructure Physics, Max Planck Institute for Solid State Research, Diamond Light Source, Muroran Institute of Technology