Zhuoyun Tang

Fe 3 d Electron Delocalization in Asymmetric Fe Single Atoms Enables Nonradical Peroxymonosulfate Activation for Micropollutant Degradation

Nonradical peroxymonosulfate (PMS) activation provides a selective route for micropollutant degradation, yet the orbital-level origin of oxidant speciation at single-atom sites remains unclear. Herein, an asymmetric Fe single-atom catalyst (Fe-N3-VN-C) is synthesized via molten-s...