Yusuke Yamauchi

Coordinating Mesopore Geometry and Interfacial Water Dynamics for Iron‐Site Evolution in Nitrate Electroreduction

ABSTRACT Developing electrocatalysts with active sites that undergo structural evolution under operating conditions remains a challenge in electrochemical nitrate reduction. Here, we use single‐crystalline mesoporous metal–organic frameworks (MOFs) with distinct pore geometries t...

Metal‐Organic Framework‐Templated Deconstruction‐Reconstruction Enables One‐Dimensional to Two‐Dimensional Self‐Assembly of Transition Metal Phosphates for High‐Performance Ammonia Sensing

ABSTRACT Self‐assembled nanomaterials formed through the spontaneous organisation of nanoscale building blocks are attractive because of their high surface areas, strong interparticle connectivity, and ease of processing. However, programming the assembly of one‐dimensional (1D)...

Electrodeposition-initiated, self-catalyzed growth of 2D amorphous Fe-group metal–boron alloy mesoporous films

Two-dimensional mesoporous amorphous metallic films, particularly those based on earth-abundant Fe-group metals (Ni, Co, Fe), are highly promising for various applications due to their high surface area, structural isotropy, and abundant undercoordinated sites. However, synthesiz...