Tianyi Gao

Spin Polarization Enables Spin-Conserved Intermediate Migration for Selective C–N Coupling toward Urea Electrosynthesis

Abstract Electrochemical coreduction of CO2 and nitrate to urea offers a promising approach to carbon–nitrogen fixation but still suffers from sluggish C–N coupling and severe competition from ammonia formation. Existing studies primarily focus on intermediate adsorption and larg...