R. J. Dwayne Miller

Controlling Nonadiabatic Transitions through Engineered Ultrafast Laser Fields at Conical Intersections

Abstract In this paper, we investigate the coherent control of nonadiabatic dynamics at a conical intersection (CI) using engineered ultrafast laser pulses. Within a model vibronic system, we tailor the pulse chirp and temporal profile and compute the resulting wave packet popula...