Oliver Millington

An Energy-GradientStrategy for Triplet-Pair Separationin Singlet-Fission Oligomers

Abstract Singlet fission (SF) offers a pathway to surpass the Shockley–Queisser limit by converting one photoexcited singlet exciton into two triplet excitons. However, in molecular assemblies, this process commonly yields a strongly exchange-coupled correlated triplet pair, 1(TT...