Mengke Zhang

Confined Predesolvation in a Yolk–Shell Metal–Organic Framework Interphase Enables Reversible Lithium-Metal Anodes

Abstract Artificial interfaces for lithium-metal anodes typically regulate nucleation after Li+ desolvation, while the preceding solvation-to-interface transition remains poorly controlled. Herein, we show that a yolk–shell H-Fe3O4@ZIF-67 interphase can act as a confined predesol...