Long Shi

A Comprehensive Enhancement of the Photochemical Properties of Metal Nanoclusters via Ligand‐Tailoring and Fluorine‐Incorporation

ABSTRACT Metal nanoclusters have garnered significant research interest over the past two decades due to their unique photochemical properties. Herein, we synthesize Au 25 nanoclusters with various previously unused surface ligands. By systematically comparing their photoinitiati...

Native Mass Spectrometry-Based Proteoform Explicit Metrics System (PrEMS) Informs Structural Improvement of Artificial Photocyclase Enzymes

Abstract Directed evolution is a powerful strategy for enzyme engineering and has successfully enabled unique stereoselective biosynthesis of high-value organic molecules. Enantiomeric excess (ee) remains the gold standard to assess the enzyme performance, but only reflects the f...