Françisco M. Raymo

Accurate and Robust Measurement of Single-Molecule Fluorescence Spectral Heterogeneity

Abstract Understanding single-molecule fluorescence spectral heterogeneity (smFLUSH) is vital for developing new probes for multidimensional super-resolution microscopy and decoding nanoscopic environments. However, traditional analysis methods distort the data and fail to distin...

Photochemical fluorescence activation in arrays of microspherical containers

Abstract Synthetic dyes with photoactivatable emission permit the photochemical control of the spatial distribution of fluorescence. When their diffusion is restricted in a host matrix, patterned illumination enables the photochemical imprinting of information in the form of pers...