Aofei Cheng

Insights on Dual‐Functional Ionic Liquid Interfacial Layer for Efficient CO 2 Electroreduction to C 2+ Products in Acid

ABSTRACT Electrocatalytic CO 2 reduction reaction (CO 2 RR) in acidic electrolyte is hindered by severe hydrogen evolution reaction (HER) and inefficient C–C coupling, leading to poor selectivity toward multicarbon (C 2+ ) products. Here, we construct a dual‐functional interfacia...

Insights on Dual‐Functional Ionic Liquid Interfacial Layer for Efficient CO 2 Electroreduction to C 2+ Products in Acid

ABSTRACT Electrocatalytic CO 2 reduction reaction (CO 2 RR) in acidic electrolyte is hindered by severe hydrogen evolution reaction (HER) and inefficient C–C coupling, leading to poor selectivity toward multicarbon (C 2+ ) products. Here, we construct a dual‐functional interfacia...

Crystallinity-Dependent Reverse Hydrogen Spillover Governs Electrochemical CO2 Reduction to Methane

Abstract The electrochemical CO2 reduction reaction (CO2RR) is a proton−electron coupled transfer process in which active hydrogen (*H) plays a pivotal role in determining the reaction pathways, particularly for methane (CH4), a representative deep hydrogenation product. However,...